{"created":"2024-07-01T02:44:36.707669+00:00","id":2001029,"links":{},"metadata":{"_buckets":{"deposit":"14e4ad82-ba5e-46d9-a3cc-744215ff9411"},"_deposit":{"created_by":17,"id":"2001029","owner":"17","owners":[17],"pid":{"revision_id":0,"type":"depid","value":"2001029"},"status":"published"},"_oai":{"id":"oai:ynu.repo.nii.ac.jp:02001029","sets":["1006:1009","495:496"]},"author_link":[],"control_number":"2001029","item_2_biblio_info_8":{"attribute_name":"書誌情報","attribute_value_mlt":[{"bibliographicIssueDates":{"bibliographicIssueDate":"2024-05-26","bibliographicIssueDateType":"Issued"},"bibliographicIssueNumber":"11","bibliographicNumberOfPages":"8","bibliographicPageEnd":"8929","bibliographicPageStart":"8922","bibliographicVolumeNumber":"14","bibliographic_titles":[{"bibliographic_title":"ACS Catalysis","bibliographic_titleLang":"en"}]}]},"item_2_description_5":{"attribute_name":"抄録","attribute_value_mlt":[{"subitem_description":"Transition metals, such as nickel (Ni), cobalt (Co), and iron (Fe), exhibit catalytic activity for electrochemical oxidation under basic conditions. In this study, we demonstrate the highly selective electrochemical oxidation of primary alcohols to aldehydes using Ni, Co, and Fe catalysts in an anion-exchange membrane (AEM) reactor. Our findings indicate that non-noble metal catalysts can be utilized for the electrocatalytic oxidation of primary alcohols by leveraging basic conditions that do not corrode these metals. In addition, we prepared binary metal alloys and oxide catalysts and investigated their catalytic abilities for alcohol oxidation. The results demonstrate that controlling the oxygen evolution reaction potential through the composition ratio of the binary catalyst and avoiding interference with the desired alcohol oxidation are crucial for increasing the yield of the oxidation products. Furthermore, despite the basic nature of the reaction sites, the electrocatalytic oxidation of primary alcohols selectively yielded the corresponding aldehydes, which was attributed to the unique triple-phase interfacial reaction sites in the AEM reactor.","subitem_description_language":"en","subitem_description_type":"Abstract"}]},"item_2_publisher_35":{"attribute_name":"出版者","attribute_value_mlt":[{"subitem_publisher":"American Chemical Society"}]},"item_2_relation_13":{"attribute_name":"DOI","attribute_value_mlt":[{"subitem_relation_type":"isVersionOf","subitem_relation_type_id":{"subitem_relation_type_id_text":"https://doi.org/10.1021/acscatal.4c01097","subitem_relation_type_select":"DOI"}}]},"item_2_rights_14":{"attribute_name":"権利","attribute_value_mlt":[{"subitem_rights":"This document is the Accepted Manuscript version of a Published Work that appeared in final form in ACS Catalysis, copyright © 2024 American Chemical Society after peer review and technical editing by the publisher. To access the final edited and published work see https://pubs.acs.org/articlesonrequest/AOR-IICZNPXUZEPIH9F6V3DQ .","subitem_rights_language":"en","subitem_rights_resource":"https://pubs.acs.org/page/copyright/journals/posting_policies.html"}]},"item_2_source_id_11":{"attribute_name":"書誌レコードID","attribute_value_mlt":[{"subitem_source_identifier":"AA12599706","subitem_source_identifier_type":"NCID"}]},"item_2_source_id_9":{"attribute_name":"ISSN","attribute_value_mlt":[{"subitem_source_identifier":"21555435","subitem_source_identifier_type":"EISSN"}]},"item_2_version_type_18":{"attribute_name":"著者版フラグ","attribute_value_mlt":[{"subitem_version_resource":"http://purl.org/coar/version/c_ab4af688f83e57aa","subitem_version_type":"AM"}]},"item_access_right":{"attribute_name":"アクセス権","attribute_value_mlt":[{"subitem_access_right":"open 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Yokohama National University","affiliationNameLang":"en"}]}],"creatorNames":[{"creatorName":"Yusuke, Muto","creatorNameLang":"en"}]},{"creatorAffiliations":[{"affiliationNames":[{"affiliationName":"Department of Chemistry and Life Science, Yokohama National University","affiliationNameLang":"en"}]}],"creatorNames":[{"creatorName":"Akizumi, Yonezawa","creatorNameLang":"en"}]},{"creatorAffiliations":[{"affiliationNames":[{"affiliationName":"Graduate School of Engineering, Kyoto University","affiliationNameLang":"en"}]}],"creatorNames":[{"creatorName":"Shoji, Iguchi","creatorNameLang":"en"}],"nameIdentifiers":[{"nameIdentifier":"0000-0002-2522-1358","nameIdentifierScheme":"ORCID","nameIdentifierURI":"https://orcid.org/0000-0002-2522-1358"}]},{"creatorAffiliations":[{"affiliationNames":[{"affiliationName":"Department of Chemistry and Life Science, Yokohama National University","affiliationNameLang":"en"}]},{"affiliationNames":[{"affiliationName":"Institute of Advanced Sciences, Yokohama National University","affiliationNameLang":"en"}]},{"affiliationNames":[{"affiliationName":"PRESTO, Japan Science and Technology Agency (JST)","affiliationNameLang":"en"}]}],"creatorNames":[{"creatorName":"Naoki, Shida","creatorNameLang":"en"}],"nameIdentifiers":[{"nameIdentifier":"0000-0003-0586-1216","nameIdentifierScheme":"ORCID","nameIdentifierURI":"https://orcid.org/0000-0003-0586-1216"}]},{"creatorAffiliations":[{"affiliationNames":[{"affiliationName":"Department of Chemistry and Life Science, Yokohama National University","affiliationNameLang":"en"}]},{"affiliationNames":[{"affiliationName":"Institute of Advanced Sciences, Yokohama National University","affiliationNameLang":"en"}]}],"creatorNames":[{"creatorName":"Mahito, Atobe","creatorNameLang":"en"}],"nameIdentifiers":[{"nameIdentifier":"0000-0002-3173-3608","nameIdentifierScheme":"ORCID","nameIdentifierURI":"https://orcid.org/0000-0002-3173-3608"}]}]},"item_files":{"attribute_name":"ファイル情報","attribute_type":"file","attribute_value_mlt":[{"accessrole":"open_date","date":[{"dateType":"Available","dateValue":"2025-05-27"}],"fileDate":[{"fileDateType":"Issued","fileDateValue":"2024-05-26"}],"filename":"Revised_manuscript_cs-2024-01097cR2.docx.pdf","filesize":[{"value":"1.7 MB"}],"format":"application/pdf","mimetype":"application/pdf","url":{"label":"Revised_manuscript_cs-2024-01097cR2.docx.pdf","objectType":"fulltext","url":"https://ynu.repo.nii.ac.jp/record/2001029/files/Revised_manuscript_cs-2024-01097cR2.docx.pdf"},"version_id":"ad161e01-1b8d-4ed4-b198-6d99aee3ca9f"}]},"item_keyword":{"attribute_name":"キーワード","attribute_value_mlt":[{"subitem_subject":"electrosynthesis, anion-exchange membrane reactor, electrocatalytic oxidation, oxyhydroxide, triple-phase boundary","subitem_subject_language":"en","subitem_subject_scheme":"Other"}]},"item_language":{"attribute_name":"言語","attribute_value_mlt":[{"subitem_language":"eng"}]},"item_resource_type":{"attribute_name":"資源タイプ","attribute_value_mlt":[{"resourcetype":"journal article","resourceuri":"http://purl.org/coar/resource_type/c_6501"}]},"item_title":"Electrocatalytic Oxidation of Primary Alcohols at the Triple-Phase Boundary in an Anion-Exchange Membrane Reactor with Nickel, Cobalt, and Iron Catalysts","item_titles":{"attribute_name":"タイトル","attribute_value_mlt":[{"subitem_title":"Electrocatalytic Oxidation of Primary Alcohols at the Triple-Phase Boundary in an Anion-Exchange Membrane Reactor with Nickel, Cobalt, and Iron Catalysts","subitem_title_language":"en"}]},"item_type_id":"2","owner":"17","path":["496","1009"],"pubdate":{"attribute_name":"PubDate","attribute_value":"2024-07-01"},"publish_date":"2024-07-01","publish_status":"0","recid":"2001029","relation_version_is_last":true,"title":["Electrocatalytic Oxidation of Primary Alcohols at the Triple-Phase Boundary in an Anion-Exchange Membrane Reactor with Nickel, Cobalt, and Iron Catalysts"],"weko_creator_id":"17","weko_shared_id":-1},"updated":"2024-07-01T04:40:39.271905+00:00"}